An illustration depicts pairs of superconducting electrons in rhombohedral graphene (the middle lattice structure) that spin in clockwise or counterclockwise direction (corresponding to blue and red colors). The electron pairs exhibit properties of magnetism and superconductivity that were not thought to co-exist in one material. The electronic state represents a new form of magnetic superconductor.
Credit: Sampson Wilcox, Research Laboratory of Electronics
MIT scientists have identified a bizarre new material: a superconductor that also acts like a magnet. Using a special stacking of graphene layers from graphite, they observed this dual behavior — something thought to be impossible until now.
For over a century, scientists believed that magnets and superconductors were fundamentally incompatible, like mixing oil with water. But a groundbreaking discovery from MIT physicists is now turning that idea on its head.
In a recent study published in Nature, the research team revealed something remarkable: a new material called a chiral superconductor. It carries electricity with zero resistance, and it’s magnetic. This strange combination has never been observed in such a direct way before.
Even more surprising? The researchers found this exotic behavior in a very familiar substance: graphite, the same material used in pencil lead.
Graphite’s Hidden Potential Unlocked
Graphite is made up of countless layers of graphene, a one-atom-thick sheet of carbon atoms arranged in a honeycomb pattern. Normally, these layers are stacked neatly on top of one another and can easily flake off when pressure is applied, as when pressing down with a pencil to write on a piece of paper. But sometimes, tiny pockets form where the stacking is slightly skewed, creating a staircase-like pattern.
MIT scientists discovered that when just four or five layers are arranged in this special “rhombohedral” pattern, the material can behave in an entirely new way—unlocking electronic properties never seen in regular graphite.
Credit: Sampson Wilcox, Research Laboratory of Electronics
Creating Superconductivity in Rhombohedral Graphene
In their new study, the physicists isolated microscopic flakes of rhombohedral graphene from graphite, and subjected the flakes to a battery of electrical tests. They found that when the flakes are cooled to 300 millikelvins (about -273 degrees Celsius), the material turns into a superconductor, meaning that any electrical current passing through the material can flow through without resistance.
They also found that when they swept an external magnetic field up and down, the flakes could be switched between two different superconducting states, just like a magnet. This suggests that the superconductor has some internal, intrinsic magnetism. Such switching behavior is absent in other superconductors.
“The general lore is that superconductors do not like magnetic fields,” says Long Ju, assistant professor of physics at MIT. “But we believe this is the first observation of a superconductor that behaves as a magnet with such direct and simple evidence. And that’s quite a bizarre thing because it is against people’s general impression on superconductivity and magnetism.”
Ju is the senior author of the study, which includes MIT co-authors Tonghang Han, Zhengguang Lu, Zach Hadjri, Lihan Shi, Zhenghan Wu, Wei Xu, Yuxuan Yao, Jixiang Yang, Junseok Seo, Shenyong Ye, Muyang Zhou, and Liang Fu, along with collaborators from Florida State University, the University of Basel in Switzerland, and the National Institute for Materials Science in Japan.
Creating Superconductivity in Rhombohedral Graphene
In their new study, the physicists isolated microscopic flakes of rhombohedral graphene from graphite, and subjected the flakes to a battery of electrical tests. They found that when the flakes are cooled to 300 millikelvins (about -273 degrees Celsius), the material turns into a superconductor, meaning that any electrical current passing through the material can flow through without resistance.
They also found that when they swept an external magnetic field up and down, the flakes could be switched between two different superconducting states, just like a magnet. This suggests that the superconductor has some internal, intrinsic magnetism. Such switching behavior is absent in other superconductors.
“The general lore is that superconductors do not like magnetic fields,” says Long Ju, assistant professor of physics at MIT. “But we believe this is the first observation of a superconductor that behaves as a magnet with such direct and simple evidence. And that’s quite a bizarre thing because it is against people’s general impression on superconductivity and magnetism.”
Ju is the senior author of the study, which includes MIT co-authors Tonghang Han, Zhengguang Lu, Zach Hadjri, Lihan Shi, Zhenghan Wu, Wei Xu, Yuxuan Yao, Jixiang Yang, Junseok Seo, Shenyong Ye, Muyang Zhou, and Liang Fu, along with collaborators from Florida State University, the University of Basel in Switzerland, and the National Institute for Materials Science in Japan.
Challenging Long-Held Superconductor Assumptions
In everyday conductive materials, electrons flow through in a chaotic scramble, whizzing by each other, and pinging off the material’s atomic latticework. Each time an electron scatters off an atom, it has, in essence, met some resistance, and loses some energy as a result, normally in the form of heat. In contrast, when certain materials are cooled to ultracold temperatures, they can become superconducting, meaning that the material can allow electrons to pair up, in what physicists term “Cooper pairs.” Rather than scattering away, these electron pairs glide through a material without resistance. With a superconductor, then, no energy is lost in translation.
Since superconductivity was first observed in 1911, physicists have shown many times over that zero electrical resistance is a hallmark of a superconductor. Another defining property was first observed in 1933, when the physicist Walther Meissner discovered that a superconductor will expel an external magnetic field. This “Meissner effect” is due in part to a superconductor’s electron pairs, which collectively act to push away any magnetic field.
Physicists have assumed that all superconducting materials should exhibit both zero electrical resistance, and a natural magnetic repulsion. Indeed, these two properties are what could enable Maglev, or “magnetic levitation” trains, whereby a superconducting rail repels and therefore levitates a magnetized car.
A Strange Twist Sparks Superconductivity
Ju and his colleagues had no reason to question this assumption as they carried out their experiments at MIT. In the last few years, the team has been exploring the electrical properties of pentalayer rhombohedral graphene. The researchers have observed surprising properties in the five-layer, staircase-like graphene structure, most recently that it enables electrons to split into fractions of themselves. This phenomenon occurs when the pentalayer structure is placed atop a sheet of hexagonal boron nitride (a material similar to graphene), and slightly offset by a specific angle, or twist.
Curious as to how electron fractions might change with changing conditions, the researchers followed up their initial discovery with similar tests, this time by misaligning the graphene and hexagonal boron nitride structures. To their surprise, they found that when they misaligned the two materials and sent an electrical current through, at temperatures less than 300 millikelvins, they measured zero resistance. It seemed that the phenomenon of electron fractions disappeared, and what emerged instead was superconductivity.
Bizarre Resistance Spikes Defy Conventional Physics
The researchers went a step further to see how this new superconducting state would respond to an external magnetic field. They applied a magnet to the material, along with a voltage, and measured the electrical current coming out of the material. As they dialed the magnetic field from negative to positive (similar to a north and south polarity) and back again, they observed that the material maintained its superconducting, zero-resistance state, except in two instances, once at either magnetic polarity. In these instances, the resistance briefly spiked, before switching back to zero, and returning to a superconducting state.
“If this were a conventional superconductor, it would just remain at zero resistance until the magnetic field reaches a critical point, where superconductivity would be killed,” Zach Hadjri, a first-year student in the group, says. “Instead, this material seems to switch between two superconducting states, like a magnet that starts out pointing upward, and can flip downwards when you apply a magnetic field. So it looks like this is a superconductor that also acts like a magnet. Which doesn’t make any sense!”
The researchers went a step further to see how this new superconducting state would respond to an external magnetic field. They applied a magnet to the material, along with a voltage, and measured the electrical current coming out of the material. As they dialed the magnetic field from negative to positive (similar to a north and south polarity) and back again, they observed that the material maintained its superconducting, zero-resistance state, except in two instances, once at either magnetic polarity. In these instances, the resistance briefly spiked, before switching back to zero, and returning to a superconducting state.
“If this were a conventional superconductor, it would just remain at zero resistance until the magnetic field reaches a critical point, where superconductivity would be killed,” Zach Hadjri, a first-year student in the group, says. “Instead, this material seems to switch between two superconducting states, like a magnet that starts out pointing upward, and can flip downwards when you apply a magnetic field. So it looks like this is a superconductor that also acts like a magnet. Which doesn’t make any sense!”
Rhombohedral Graphene’s Quantum Secrets
As counterintuitive as the discovery may seem, the team observed the same phenomenon in six similar samples. They suspect that the unique configuration of rhombohedral graphene is the key. The material has a very simple arrangement of carbon atoms. When cooled to ultracold temperatures, the thermal fluctuation is minimized, allowing any electrons flowing through the material to slow down, sense each other, and interact.
Such quantum interactions can lead electrons to pair up and superconduct. These interactions can also encourage electrons to coordinate. Namely, electrons can collectively occupy one of two opposite momentum states, or “valleys.” When all electrons are in one valley, they effectively spin in one direction, versus the opposite direction. In conventional superconductors, electrons can occupy either valley, and any pair of electrons is typically made from electrons of opposite valleys that cancel each other out. The pair overall then, has zero momentum, and does not spin.
In the team’s material structure, however, they suspect that all electrons interact such that they share the same valley, or momentum state. When electrons then pair up, the superconducting pair overall has a “non-zero” momentum, and spinning, that, along with many other pairs, can amount to an internal, superconducting magnetism.
Theoretical Implications and Quantum Computing Potential
“You can think of the two electrons in a pair spinning clockwise, or counterclockwise, which corresponds to a magnet pointing up, or down,” Tonghang Han, a fifth-year student in the group, explains. “So we think this is the first observation of a superconductor that behaves as a magnet due to the electrons’ orbital motion, which is known as a chiral superconductor. It’s one of a kind. It is also a candidate for a topological superconductor which could enable robust quantum computation.”
“Everything we’ve discovered in this material has been completely out of the blue,” says Zhengguang Lu, a former postdoc in the group and now an assistant professor at Florida State University. “But because this is a simple system, we think we have a good chance of understanding what is going on, and could demonstrate some very profound and deep physics principles.”
“It is truly remarkable that such an exotic chiral superconductor emerges from such simple ingredients,” adds Liang Fu, professor of physics at MIT. “Superconductivity in rhombodedral graphene will surely have a lot to offer.”
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